Pumps don't really need to "chill". You don't want the pump cycling on and off when water is being used. The pump needs to run continuously while any water is being used, then it can "chill" when no water is running.
If you can live with 35 GPM at 50 PSI up top, then you need to run a 60/80 pressure switch and a 70 PSI CSV at the bottom. The problem is that pump cannot afford any friction loss or reduced pressure fall off as comes with the CSV2W. The CSV3B2T is a little overkill for that size pump, but that is the reason it won't have the friction loss of the smaller CSV2W.
I would run a CSV3B2T set at 70 PSI, with a 60/80 GHG pressure switch on at least a 44 gallon size tank. You can go larger with the pressure tank is you want, but the smaller tank will be fine, and it will offset some of the cost of the CSV3B2T which sells for $647.50.